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Screening the emission sources of volatile organic compounds (VOCs) in China by multi-effects evaluation

He NIU,Ziwei MO,Min SHAO,Sihua LU,Shaodong XIE

《环境科学与工程前沿（英文）》 2016年 第10卷 第5期 doi: 10.1007/s11783-016-0828-z

摘要： We develop a multi-effect evaluation method to assess integrated impact of VOCs. Enable policy-makers to identify important emission sources, regions, and key species. Solvent usage and industrial process are the most important anthropogenic sources. Styrene, toluene, ethylene, benzene, and m/p-xylene are key species to be cut. Volatile organic compounds (VOCs) play important roles in the atmosphere via three main pathways: photochemical ozone formation, secondary organic aerosol production, and direct toxicity to humans. Few studies have integrated these effects to prioritize control measures for VOCs sources. In this study, we developed a multi-effects evaluation methodology based on updated emission inventories and source profiles, by combining the ozone formation potential (OFP), secondary organic aerosol potential (SOAP), and VOC toxicity data. We derived species-specific emission inventories for 152 sources. The OFPs, SOAPs, and toxicity of each source were estimated, the contribution and sharing of source to each of these adverse effects were calculated. Weightings were given to the three adverse effects by expert scoring, and then the integrated effect was determined. Taking 2012 as the base year, solvent use and industrial process were found to be the most important anthropogenic sources, accounting for 24.2% and 23.1% of the integrated effect, respectively, followed by biomass burning, transportation, and fossil fuel combustion, each had a similar contribution ranging from 16.7% to 18.6%. The top five industrial sources, including plastic products, rubber products, chemical fiber products, the chemical industry, and oil refining, accounted for nearly 70.0% of industrial emissions. Beijing, Chongqing, Shanghai, Jiangsu, and Guangdong were the five provinces contributing the largest integrated effects. For the VOC species from emissions showed the largest contributions were styrene, toluene, ethylene, benzene, and m/p-xylene.

关键词： Ozone formation     Secondary organic aerosol     Multi-effects evaluation     VOC abatement strategy    

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A review on application of dielectric barrier discharge plasma technology on the abatement of volatile

Wenjing Lu, Yawar Abbas, Muhammad Farooq Mustafa, Chao Pan, Hongtao Wang

《环境科学与工程前沿（英文）》 2019年 第13卷 第2期 doi: 10.1007/s11783-019-1108-5

摘要：

• Applications of non-thermal plasma reactors for reduction of VOCs were reviewed.

• Dielectric barrier discharge (DBD) plasma was considered.

• Effect of process parameters was studied.

• Effect of catalysts and inhibitors were evaluated.

关键词： Non-thermal plasma (NTP)     Dielectric barrier discharge (DBD)     Volatile organic compounds (VOCs)     Abatement     Input power    

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Impact of photocatalytic remediation of pollutants on urban air quality

Christian GEORGE, Anne BEELDENS, Fotios BARMPAS, Jean-François DOUSSIN, Giuseppe MANGANELLI, Hartmut HERRMANN, Jörg KLEFFMANN, Abdelwahid MELLOUKI

《环境科学与工程前沿（英文）》 2016年 第10卷 第5期 doi: 10.1007/s11783-016-0834-1

摘要： Air pollution remediation using photocatalytic construction materials was tested. NO and VOC uptake rates on different materials were measured in the laboratory. Effective NO and VOC abatement levels were tested under real conditions. Recommendations for implementation of photocatalytic materials are provided. In the recent years, photocatalytic self-cleaning and “depolluting” materials have been suggested as a remediation technology mainly for NO and aromatic VOCs in urban areas. A number of products incorporating the aforementioned technology have been made commercially available with the aim to improve urban air quality. These commercial products are based on the photocatalytic properties of a thin layer of TiO at the surface of the material (such as glass, pavement, etc.) or embedded in paints or concrete. The use of TiO photocatalysts as an emerging air pollution control technology has been reported in many locations worldwide. However, up to now, the effectiveness measured in situ and the expected positive impact on air quality of this relatively new technology has only been demonstrated in a limited manner. Assessing and demonstrating the effectiveness of these depolluting techniques in real scale applications aims to create a real added value, in terms of policy making (i.e., implementing air quality strategies) and economics (by providing a demonstration of the actual performance of a new technique).

关键词： Photocatalysis     Air pollution     Depollution efficiency     NOx     VOC     Air quality abatement and management    

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Achieving air pollutant emission reduction targets with minimum abatement costs: An enterprise-level

《环境科学与工程前沿（英文）》 2022年 第16卷 第2期 doi: 10.1007/s11783-021-1459-6

摘要：

• Quantification of efficiency and fairness of abatement allocation are optimized.

关键词： Pollutant emission reduction allocation     Emission reduction measures     Total abatement cost     Economic efficiency     Abatement space    

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The abatement of major pollutants in air and water by environmental catalysis

Junhua LI, Hong HE, Chun HU, Jincai ZHAO

《环境科学与工程前沿（英文）》 2013年 第7卷 第3期   页码 302-325 doi: 10.1007/s11783-013-0511-6

摘要： This review reports the research progress in the abatement of major pollutants in air and water by environmental catalysis. For air pollution control, the selective catalytic reduction of NO (SCR) by ammonia and hydrocarbons on metal oxide and zeolite catalysts are reviewed and discussed, as is the removal of Hg from flue gas by catalysis. The oxidation of Volatile organic compounds (VOCs) by photo- and thermal- catalysis for indoor air quality improvement is reviewed. For wastewater treatment, the catalytic elimination of inorganic and organic pollutants in wastewater is presented. In addition, the mechanism for the procedure of abatement of air and water pollutants by catalysis is discussed in this review. Finally, a research orientation on environment catalysis for the treatment of air pollutants and wastewater is proposed.

关键词： air pollution control     wastewater treatment     DeNOx     selective catalytic reduction (SCR)     Volatile organic compounds (VOCs)     environmental catalysis    

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Construction of MOFs-based nanocomposite membranes for emerging organic contaminants abatement in water

《环境科学与工程前沿（英文）》 2023年 第17卷 第7期 doi: 10.1007/s11783-023-1689-x

摘要：

● Application of the MOF-composite membranes in adsorption was discussed.

关键词： Emerging organic contaminants     Metal organic frameworks     Synthesis     Adsorption     Catalysis    

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Process simulation and economic analysis of reactor systems for perfluorinated compounds abatement without

Boreum Lee,Sunggeun Lee,Ho Young Jung,Shin-Kun Ryi,Hankwon Lim

《化学科学与工程前沿（英文）》 2016年 第10卷 第4期   页码 526-533 doi: 10.1007/s11705-016-1590-2

摘要： New and efficient reactor systems were proposed to treat perfluorinated compounds via catalytic decomposition. One system has a single reactor (S-1), and another has a series of reactors (S-2). Both systems are capable of producing a valuable CaF and eliminating toxic HF effluent and their feasibility was studied at various temperatures with a commercial process simulator, Aspen HYSYS . They are better than the conventional system, and S-2 is better than S-1 in terms of CaF production, a required heat for the system, natural gas usage and CO emissions in a boiler, and energy consumption. Based on process simulation results, preliminary economic analysis shows that cost savings of 12.37% and 13.55% were obtained in S-2 at 589.6 and 621.4 °C compared to S-1 at 700 and 750 °C, respectively, for the same amount of CaF production.

关键词： perfluorinated compounds (PFCs)     CF4     process simulation     economic analysis    

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Integration of molecular dynamic simulation and free volume theory for modeling membrane VOC/gas separation

Bo Chen, Yan Dai, Xuehua Ruan, Yuan Xi, Gaohong He

《化学科学与工程前沿（英文）》 2018年 第12卷 第2期   页码 296-305 doi: 10.1007/s11705-018-1701-3

摘要： Gas membrane separation process is highly unpredictable due to interacting non-ideal factors, such as composition/pressure-dependent permeabilities and real gas behavior. Although molecular dynamic (MD) simulation can mimic those complex effects, it cannot precisely predict bulk properties due to scale limitations of calculation algorithm. This work proposes a method for modeling a membrane separation process for volatile organic compounds by combining the MD simulation with the free volume theory. This method can avoid the scale-up problems of the MD method and accurately simulate the performance of membranes. Small scale MD simulation and pure gas permeation data are employed to correlate pressure-irrelevant parameters for the free volume theory; by this approach, the microscopic effects can be directly linked to bulk properties (non-ideal permeability), instead of being fitted by a statistical approach. A lab-scale hollow fiber membrane module was prepared for the model validation and evaluation. The comparison of model predictions with experimental results shows that the deviations of product purity are reduced from 10% to less than 1%, and the deviations of the permeate and residue flow rates are significantly reduced from 40% to 4%, indicating the reliability of the model. The proposed method provides an efficient tool for process engineering to simulate the membrane recovery process.

关键词： membrane vapor separation     membrane process modeling     process engineering     free volume theory     volatile organic compound    

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Suspended solid abatement in a conical fluidized bed flocculator

Dandan ZHOU, Shuangshi DONG, Keyu LI, Huizhong JIANG, Dandan SHANG

《环境科学与工程前沿（英文）》 2013年 第7卷 第1期   页码 127-134 doi: 10.1007/s11783-012-0415-x

摘要： With the random movement of silica gel beads in a conical fluidized bed, micro-vortices resulting from the fluidization promoted the collision and aggregation of suspended fine kaolin powders. The abatement efficiencies of the suspended fine solids under several hydrodynamic conditions were studied, and a suitable control strategy for operating the conical fluidized bed flocculators was identified. The suspended solids abatement efficiency was found to increase with increasing Camp Number and flocculation time ( ), but decreased with the increase of velocity gradient ( ) within the range studied in this research (165.1–189.6 s ). The abatement efficiencies were all more than 60% at the range of = 165–180 s and = 15–33 s at an initial kaolin solid concentration of 150 mg·L , polymer aluminum chloride dosage of 60 mg·L and sedimentation time of 20 min. However, the formation of flocs was influenced by the liquid backmixing. Excessive backmixing caused the breakup of flocs and resulted in difficulty for the fine powders to aggregate and sediment to the reactor bottom. The results of the calculated fractal dimension and measured free sedimentation velocity of flocs obtained at different runs showed similar flocs properties, and indicated an easy control strategy for sedimentation of the flocs.

关键词： conical fluidized bed     flocculation     velocity gradient    

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Tailoring the simultaneous abatement of methanol and NO on Sb-Ce-Zr catalysts via copper modification

《环境科学与工程前沿（英文）》 2022年 第16卷 第10期 doi: 10.1007/s11684-022-1565-0

摘要：

● Cu addition enhances CH3OH oxidation and alleviates its inhibitory effect on SCR.

关键词： Copper modification     Sb-CeZr2Ox catalyst     NOx     Methanol     Simultaneous removal    

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生物法净化低浓度挥发性有机废气研究

杨显万,孙珮石,黄若华,黄兵,陈茂生

《中国工程科学》 2001年 第3卷 第9期   页码 64-68

摘要：

以低浓度甲苯（VOC）废气为对象，对生物法有机废气净化技术进行了小试、扩试与工业试验的系 统研究。

关键词： 生物法VOC废气净化技术     甲苯生化降解     吸附-生物膜理论     工业应用试验    

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Magnetic Co-doped 1D/2D structured -FeO/MoS effectively activated peroxymonosulfate for efficient abatement

《环境科学与工程前沿（英文）》 2023年 第18卷 第3期 doi: 10.1007/s11783-024-1797-2

摘要：

● Magnetic Co- γ -Fe2O3/MoS2 were prepared via facile hydrothermal methods.

关键词： Magnetic Co-γ-Fe2O3/MoS2     Hydrothermal method     Bisphenol A     Degradation pathways     Toxicity analysis    

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Impacts of emissions and meteorological changes on China’s ozone pollution in the warm seasons of 2013 and 2017

Dian Ding, Jia Xing, Shuxiao Wang, Xing Chang, Jiming Hao

《环境科学与工程前沿（英文）》 2019年 第13卷 第5期 doi: 10.1007/s11783-019-1160-1

摘要： O3 increment is mainly caused by changes in meteorology rather than emissions. Emission reduction is effective to reduce O3 nationwide, especially in summer. Strengthened NOx controls are necessary to meet the ambient O3 standard. We have quantified the impacts of anthropogenic emissions reductions caused by the Air Pollution Control Action Plan and changes in meteorological fields between 2013 and 2017 on the warm-season O3 concentration in China using a regional 3D chemical transport model. We found that the impact on daily maximum eight-hour (MDA8) O3 concentration by the meteorological variation that mostly increased O3 was greater than that from emission reduction, which decreased O3. Specifically, the control measures implemented since 2013 in China have reduced SO2, NOx, PM2.5, and VOC emissions by 33%, 25%, 30%, and 4% in 2017, while NH3 emissions have increased by 7%. The changes in anthropogenic emissions lowered MDA8 O3 by 0.4–3.7 ppb (0.8%–7.6%, varying by region and month), although MDA8 O3 was increased slightly in some urban areas (i.e. North China) at the beginning/end of warm seasons. Relative to 2013, the average 2 m temperature in 2017 shows increments in North, North-east, East, and South China (0.34℃–0.83℃) and decreases in Central China (0.24℃). The average solar radiation shows increments in North, North-east, and South China (7.0–9.7 w/m2) and decreases in Central, South-west, and North-west China (4.7–10.3 w/m2). The meteorological differences significantly change MDA8 O3 by -3.5–8.5 ppb (-8.2%–18.8%) with large temporal variations. The average MDA8 O3 was slightly increased in North, North-east, East, and South China. The response surface model suggests that the O3 formation regime transfers from NOx-saturated in April to NOx-limited in July on average in China.

关键词： O3 pollution     Meteorological influences     Emission reduction     NOx     VOC    

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Room temperature oxidation of acetone by ozone over alumina-supported manganese and cobalt mixed oxides

Mehraneh Ghavami, Mostafa Aghbolaghy, Jafar Soltan, Ning Chen

《化学科学与工程前沿（英文）》 2020年 第14卷 第6期   页码 937-947 doi: 10.1007/s11705-019-1900-6

摘要： Volatile organic compounds (VOCs) are among the major sources of air pollution. Catalytic ozonation is an efficient process for removing VOCs at lower reaction temperature compared to catalytic oxidation. In this study, a series of alumina supported single and mixed manganese and cobalt oxides catalysts were used for ozonation of acetone at room temperature. The influence of augmenting the single Mn and Co catalysts were investigated on the performance and structure of the catalyst. The manganese and cobalt single and mixed oxides catalysts of the formula Mn10%-CoX and Co10%-MnX (where X= 0, 2.5%, 5%, or 10%) were prepared. It was found that addition of Mn and Co at lower loading levels (2.5% or 5%) to single metal oxide catalysts enhanced the catalytic activity. The mixed oxides catalysts of (Mn10%-Co2.5%) and (Mn10%-Co5%) led to acetone conversion of about 84%. It is concluded that lower oxidation state of the secondary metal improves ozone decomposition and oxidation of acetone.

关键词： ozone     VOC     manganese oxides     cobalt oxides     alumina support    

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Energy efficiency and carbon dioxide emissions reduction opportunities in district heating source in Tianjin

Gaofeng CHEN, Xuejing ZHENG, Lin CONG

《能源前沿（英文）》 2012年 第6卷 第3期   页码 285-295 doi: 10.1007/s11708-012-0197-7

摘要： Building a trading market can promote energy conservation provided that the trading method is determined. Energy consumption for heat supply is huge. Tianjin Municipal Government is planning to establish an energy efficiency trading platform for district heating taking into consideration the experience in carbon trading market and specific situation in Tianjin. This paper presented an in-depth analysis of the district heating industry in Tianjin municipality, and identified the potentials of energy saving and carbon dioxide emissions reduction. Since energy efficiency was closely related to different heating source technologies, baselines were determined for boiler plants and thermal power plants respectively. Three scenarios were discussed for baseline determination. 472 boiler plants were surveyed and operational data relating to energy consumption were collected. Through data analysis, 27 boiler plants which have reasonable recorded energy consumption values were chosen as samples. By analyzing the dataset and referring to the related standards, method of determining the baseline for district heating carbon market was established. Finxally, the baseline for boiler plant was determined to be 52.0 kgce/GJ, and that for thermal power plant was 43.0 kgce/GJ in 2011. Carbon abatement against the baselines above was calculated and considerable carbon dioxide emissions reduction could be achieved.

关键词： district heating     energy efficiency     baseline     carbon abatement    

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标题 作者 时间 类型 操作

Screening the emission sources of volatile organic compounds (VOCs) in China by multi-effects evaluation

He NIU,Ziwei MO,Min SHAO,Sihua LU,Shaodong XIE

期刊论文

A review on application of dielectric barrier discharge plasma technology on the abatement of volatile

Wenjing Lu, Yawar Abbas, Muhammad Farooq Mustafa, Chao Pan, Hongtao Wang

期刊论文

Impact of photocatalytic remediation of pollutants on urban air quality

Christian GEORGE, Anne BEELDENS, Fotios BARMPAS, Jean-François DOUSSIN, Giuseppe MANGANELLI, Hartmut HERRMANN, Jörg KLEFFMANN, Abdelwahid MELLOUKI

期刊论文

Achieving air pollutant emission reduction targets with minimum abatement costs: An enterprise-level

期刊论文

The abatement of major pollutants in air and water by environmental catalysis

Junhua LI, Hong HE, Chun HU, Jincai ZHAO

期刊论文

Construction of MOFs-based nanocomposite membranes for emerging organic contaminants abatement in water

期刊论文

Process simulation and economic analysis of reactor systems for perfluorinated compounds abatement without

Boreum Lee,Sunggeun Lee,Ho Young Jung,Shin-Kun Ryi,Hankwon Lim

期刊论文

Integration of molecular dynamic simulation and free volume theory for modeling membrane VOC/gas separation

Bo Chen, Yan Dai, Xuehua Ruan, Yuan Xi, Gaohong He

期刊论文

Suspended solid abatement in a conical fluidized bed flocculator

Dandan ZHOU, Shuangshi DONG, Keyu LI, Huizhong JIANG, Dandan SHANG

期刊论文

Tailoring the simultaneous abatement of methanol and NO on Sb-Ce-Zr catalysts via copper modification

期刊论文

生物法净化低浓度挥发性有机废气研究

杨显万,孙珮石,黄若华,黄兵,陈茂生

期刊论文

Magnetic Co-doped 1D/2D structured -FeO/MoS effectively activated peroxymonosulfate for efficient abatement

期刊论文

Impacts of emissions and meteorological changes on China’s ozone pollution in the warm seasons of 2013 and 2017

Dian Ding, Jia Xing, Shuxiao Wang, Xing Chang, Jiming Hao

期刊论文

Room temperature oxidation of acetone by ozone over alumina-supported manganese and cobalt mixed oxides

Mehraneh Ghavami, Mostafa Aghbolaghy, Jafar Soltan, Ning Chen

期刊论文

Energy efficiency and carbon dioxide emissions reduction opportunities in district heating source in Tianjin

Gaofeng CHEN, Xuejing ZHENG, Lin CONG

期刊论文